光催化降解有机污染物技术因利用绿色环保的太阳能而备受关注,然而,光催化半导体材料光生载流子的快速复合限制了其应用。近年来,通过压电效应协同光催化技术,有望解决这一问题,从而成为新的研究热点。主要介绍了压电效应协同光催化技术的基本原理和产生压电效应的方法,以及常见的压电光催化材料降解有机污染物的研究现状。最后,对压电效应协同光催化技术降解有机污染物的研究趋势及挑战进行了展望。
The photocatalytic degradation of organic pollutants technology has attracted much attention because of the use of green and environmentally friendly solar energy sources,but the rapid recombination of photogenerated carriers of photocatalytic semiconductor materials limits its application.In recent years,the synergistic technology of piezoelectric effect and photocatalysis is expected to solve this problem,which has become a new research hotspot.This paper mainly introduced the basic principles of piezoelectric effect synergistic photocatalysis technology and the methods of generating piezoelectric effect,as well as the research status of common piezoelectric photocatalytic materials to degrade organic pollutants.Finally,the research trends and challenges of piezoelectric effect synergistic photocatalytic technology for the degradation of organic pollutants were prospected.
[1] Clarke B O,Anumol T,Barlaz M,et al.Investigating landfill leachate as a source of trace organic pollutants[J].Chemosphere,2015,127:269-275.
[2] Martínez-Escudero C M,Garrido I,Flores P,et al.Remediation of triazole,anilinopyrimidine,strobilurin and neonicotinoid pesticides in polluted soil using ozonation and solarization[J].Journal of Environmental Management,2022,310:114781.
[3] Timofeeva S S,Bodienkova G M.3rd international scientific conference on sustainable and efficient use of energy,water and natural resources19-24th April 2021[C].St Petersburg:Russian Federation,2021.
[4] Wang K Y,Wu J G,Zhao X Y.Review of measurement technologies for air pollutants at livestock and poultry farms[J].Scientia Agricultura Sinica,2019,52(8):1458-1474.
[5] Huang L,Li M,Ngo H H,et al.Spectroscopic characteristics of dissolved organic matter from aquaculture wastewater and its interaction mechanism to chlorinated phenol compound[J].Journal of Molecular Liquids,2018,263:422-427.
[6] Chong M N,Jin B,Chow C W K,et al.Recent developments in photocatalytic water treatment technology:a review[J].Water Research,2010,44(10):2997-3027.
[7] Yang J,Wang D,Han H,et al.Roles of cocatalysts in photocatalysis and photoelectrocatalysis[J].Accounts of Chemical Research,2013,46(8):1900-1909.
[8] Khaki M R D,Shafeeyan M S,Raman A A A,et al.application of doped photocatalysts for organic pollutant degradation-a review[J].Journal of Environmental Management,2017,198:78-94.
[9] He X,Kai T,Ding P.Heterojunction photocatalysts for degradation of the tetracycline antibiotic:a review[J].Environmental Chemistry Letters,2021,19(6):4563-4601.
[10] Lu Q,Wei Z,Li C,et al.Photocatalytic degradation of methyl orange by noble metal Ag modified semiconductor Zn2SnO4[J].Materials Science in Semiconductor Processing,2022,138:106290.
[11] Alhokbany N,Ahamad T,Alshehri S M.Fabrication of highly porous ZnO/Ag2O nanoparticles embedded in N-doped graphitic carbon for photocatalytic degradation of tetracycline[J].Journal of Environmental Chemical Engineering,2022,10(3):107681.
[12] Oluwasogo D A,Varangane S,Prabhu Y T,et al.Biosynthetic modulation of carbon-doped ZnO for rapid photocatalytic endocrine disruptive remediation and hydrogen evolution[J].Journal of Cleaner Production,2023,394:136393.
[13] Ni S,Fu Z,Li L,et al.Step-scheme heterojunction g-C3N4/TiO2 for efficient photocatalytic degradation of tetracycline hydrochloride under UV light[J].Colloids and Surfaces A:Physicochemical and Engineering Aspects,2022,649:129475.
[14] Bera B,Sarkar M D.Piezoelectric effect,piezotronics and piezophototronics:a review[J].Imperial Journal of Interdisciplinary Research (IJIR),2016,2(11):1407-1410.
[15] Liu L,Zhong S,Zhang L,et al.Ti doped BiOCl nanowires for piezoelectric photocatalytic degradation of organic pollutants[J].Catalysis Communications,2022,170:106493.
[16] Zhou L,Dai S,Xu S,et al.Piezoelectric effect synergistically enhances the performance of Ti32-oxo-cluster/BaTiO3/CuS pn heterojunction photocatalytic degradation of pollutants[J].Applied Catalysis B:Environmental,2021,291:120019.
[17] Metzger W K,Ahrenkiel R K,Dashdorj J,et al.Analysis of charge separation dynamics in a semiconductor junction[J].Physical Review B,2005,71(3):035301.
[18] Zhu D,Zhou Q.Action and mechanism of semiconductor photocatalysis on degradation of organic pollutants in water treatment:a review[J].Environmental Nanotechnology,Monitoring & Management,2019,12:100255.
[19] Jiang Z,Tan X,Huang Y.Piezoelectric effect enhanced photocatalysis in environmental remediation:state-of-the-art techniques and future scenarios[J].Science of the Total Environment,2022,806:150924.
[20] Zhou X,Shen B,Lyubartsev A,et al.Semiconducting piezoelectric heterostructures for piezo-and piezophotocatalysis[J].Nano Energy,2022:107141.
[21] Liu Y L,Wu J M.Synergistically catalytic activities of BiFeO3/TiO2 core-shell nanocomposites for degradation of organic dye molecule through piezophototronic effect[J].Nano Energy,2019,56:74-81.
[22] Su R,Hsain H A,Wu M,et al.Nano-ferroelectric for high efficiency overall water splitting under ultrasonic vibration[J].Angewandte Chemie International Edition,2019,58(42):15076-15081.
[23] Feng Y,Li H,Ling L,et al.Enhanced photocatalytic degradation performance by fluid-induced piezoelectric field[J].Environmental Science & Technology,2018,52(14):7842-7848.
[24] Yamagata Y,Higuchi T,Nakamura N,et al.A micro mobile mechanism using thermal expansion and its theoretical analysis.a comparison with impact drive mechanism using piezoelectric elements[C].Proceedings IEEE Micro Electro Mechanical,1994:142-147.
[25] Xu Q,Nakajima M,Ichikawa S,et al.A comparative study of microbubble generation by mechanical agitation and sonication[J].Innovative Food Science & Emerging Technologies,2008,9(4):489-494.
[26] Cafarelli A,Marino A,Vannozzi L,et al.Piezoelectric nanomaterials activated by ultrasound:the pathway from discovery to future clinical adoption[J].ACS Nano,2021,15(7):11066-11086.
[27] Amiri O,Salar K,Othman P,et al.Purification of wastewater by the piezo-catalyst effect of PbTiO3 nanostructures under ultrasonic vibration[J].Journal of Hazardous Materials,2020,394:122514.
[28] Zhang C,Lei D,Xie C,et al.Piezo-photocatalysis over metal-organic frameworks:promoting photocatalytic activity by piezoelectric effect[J].Advanced Materials,2021,33(51):2106308.
[29] Nie G,Hu K,Ren W,et al.Mechanical agitation accelerated ultrasonication for wastewater treatment:sustainable production of hydroxyl radicals[J].Water Research,2021,198:117124.
[30] Goel S,Kumar B.A review on piezo-/ferro-electric properties of morphologically diverse ZnO nanostructures[J].Journal of Alloys and Compounds,2020,816:152491.
[31] Lin H Y,Le K T,Chen P H,et al.Systematic investigation of the piezocatalysis-adsorption duality of polymorphic MoS2 nanoflowers[J].Applied Catalysis B:Environmental,2022,317:121717.
[32] Jiang W,Cai W,Lin Z,et al.Effects of Nd-doping on optical and photovoltaic properties of barium titanate thin films prepared by sol-gel method[J].Materials Research Bulletin,2013,48(9):3092-3097.
[33] Zhai T,Fang X,Liao M,et al.A comprehensive review of one-dimensional metal-oxide nanostructure photodetectors[J].Sensors,2009,9(8):6504-6529.
[34] Wang Z L.Novel nanostructures of ZnO for nanoscale photonics,optoelectronics,piezoelectricity,and sensing[J].Applied Physics A,2007,88:7-15.
[35] Wang Z L.From nanogenerators to piezotronics—a decade-long study of ZnO nanostructures[J].MRS Bulletin,2012,37(9):814-827.
[36] Ning X,Hao A,Cao Y,et al.Effective promoting piezocatalytic property of zinc oxide for degradation of organic pollutants and insight into piezocatalytic mechanism[J].Journal of Colloid and Interface Science,2020,577:290-299.
[37] Ma J,Ren J,Jia Y,et al.High efficiency bi-harvesting light/vibration energy using piezoelectric zinc oxide nanorods for dye decomposition[J].Nano Energy,2019,62:376-383.
[38] Fan H,Jiang T,Li H,et al.Effect of BiVO4 crystalline phases on the photoinduced carriers behavior and photocatalytic activity[J].The Journal of Physical Chemistry C,2012,116(3):2425-2430.
[39] Wang F,Zhang J,Jin C C,et al.Unveiling the effect of crystal facets on piezo-photocatalytic activity of BiVO4[J].Nano Energy,2022,101:107573.
[40] Kumar M,Vaish R,ben Ahmed S.Piezo-photocatalytic activity of mechanochemically synthesized BiVO4 for dye cleaning[J].Journal of the American Ceramic Society,2022,105(3):2309-2322.
[41] Wang J,Zhao B,Wang C.TiO2/KNbO3 nanocomposite for enhanced humidity sensing performance[J].Sensors and Actuators A:Physical,2023,349:114057.
[42] Liu Q,Zhan F,Luo H,et al.Mechanism of interface engineering for ultrahigh piezo-photoelectric catalytic coupling effect of BaTiO3@TiO2 microflowers[J].Applied Catalysis B:Environmental,2022,318:121817.
[43] Liu X,Xiao L,Zhang Y,et al.Significantly enhanced piezo-photocatalytic capability in BaTiO3 nanowires for degrading organic dye[J].Journal of Materiomics,2020,6(2):256-262.
[44] Singh S,Khare N.Coupling of piezoelectric,semiconducting and photoexcitation properties in NaNbO3 nanostructures for controlling electrical transport:realizing an efficient piezo-photoanode and piezo-photocatalyst[J].Nano Energy,2017,38:335-341.
[45] 李颖楷,罗睿杰,赵志成.钛酸铋钠纳米球的压电催化降解RhB性能的研究[J].广东化工,2021,48(23):1-3.
[46] 雷华.光能/机械能协同催化消除有机污染物的研究[D].杭州:浙江理工大学,2021.
[47] Li X,Qiu J,Chen X,et al.High in-plane piezoelectricity of two-dimensional Janus BiOX (X= Cl,Br,and I) monolayers[J].Materials Letters,2022,325:132867.
[48] Ismail M,Wu Z,Zhang L,et al.High-efficient synergy of piezocatalysis and photocatalysis in bismuth oxychloride nanomaterial for dye decomposition[J].Chemosphere,2019,228:212-218.
[49] Jia S,Su Y,Zhang B,et al.Few-layer MoS2nanosheet-coated KNbO3 nanowire heterostructures:piezo-photocatalytic effect enhanced hydrogen production and organic pollutant degradation[J].Nanoscale,2019,11(16):7690-7700.
[50] 杨流海,李庆明,杨华.压电诱导内建电场增强ZnO/MoS2光催化性能研究[J].化工新型材料,2021,49(S1):238-242.
[51] You H,Wu Z,Jia Y,et al.High-efficiency and mechano-/photo-bi-catalysis of piezoelectric-ZnO@photoelectric-TiO2 core-shell nanofibers for dye decomposition[J].Chemosphere,2017,183:528-535.
[52] Bai Y,Zhao J,Li Y,et al.Preparation and photocatalytic performance of TiO2/PbTiO3 fiber composite enhanced by external force induced piezoelectric field[J].Journal of the American Ceramic Society,2019,102(9):5415-5423.
[53] Feng Y,Li H,Ling L,et al.Enhanced photocatalytic degradation performance by fluid-induced piezoelectric field[J].Environmental Science & Technology,2018,52(14):7842-7848.
[54] Chen Y,Deng X,Wen J,et al.Piezo-promoted the generation of reactive oxygen species and the photodegradation of organic pollutants[J].Applied Catalysis B:Environmental,2019,258:118024.
[55] Shi Q,Zhang M,Zhang Z,et al.Energy and separation optimization of photogenerated charge in BiVO4 quantum dots by piezo-potential for efficient gaseous pollutant degradation[J].Nano Energy,2020,69:104448.
基金资助
河北省自然科学基金钢铁联合基金(E2021209002);唐山市科技局项目(21130211D;22130215H);华北理工大学省属高校基本科研业务费项目(JQN2023009)