基于全无机CsPbBr3钙钛矿太阳能电池的光电性能研究

王传坤, 郝艳玲, 张星, 陆成伟

化工新型材料 ›› 2024, Vol. 52 ›› Issue (3) : 128 -133.

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化工新型材料 ›› 2024, Vol. 52 ›› Issue (3) : 128-133. DOI: 10.19817/j.cnki.issn1006-3536.2024.03.038
新材料与新技术

基于全无机CsPbBr3钙钛矿太阳能电池的光电性能研究

    王传坤, 郝艳玲, 张星, 陆成伟
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Study on photoelectric performance of all-inorganic CsPbBr3 perovskite solar cells

  • Wang Chuankun, Hao Yanling, Zhang Xing, Lu Chengwei
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摘要

钙钛矿太阳能电池具有制作工艺简单和光电转换效率高等优点,成为光伏领域研究的热点。而全无机钙钛矿太阳能材料CsPbBr3具有较强的稳定性,是具有竞争力的钙钛矿光吸收材料。主要利用SCAPS-1D软件构建了FTO/TiO2/CsPbBr3/Cu2ZnSnS4(CZTS)/Ag平面异质结结构。研究了全无机钙钛矿材料CsPbBr3厚度和带隙对钙钛矿太阳能电池的影响。

Abstract

Perovskite solar cells have the advantages such as simple manufacturing process and high photoelectric conversion efficiency,which has become a hot spot in the field of photovoltaic research.All-inorganic perovskite material CsPbBr3 is a competitive material for perovskite light-absorbing materials due to its strong stability.In this paper,FTO/TiO2/CsPbBr3/Cu2ZnSnS4(CZTS)/Ag planar heterojunction structure was constructed by the SCAPS-1D software.The influence of the thickness and band gap of all-inorganic perovskite material CsPbBr3 on perovskite solar cells was studied.

关键词

钙钛矿太阳能电池 / 全无机CsPbBr3 / 带隙 / 光电转换效率

Key words

perovskite solar cells / all-inorganic CsPbBr3 / band gap / photoelectric conversion efficiency

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基于全无机CsPbBr3钙钛矿太阳能电池的光电性能研究[J]. 化工新型材料, 2024, 52(3): 128-133 DOI:10.19817/j.cnki.issn1006-3536.2024.03.038

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参考文献

[1] Jung H S,Park N G.Perovskite solar cells:from materials to devices[J].Small,2015,11(1):10-25.
[2] Rong Y,Hu Y,Mei A,et al.Challenges for commercializing perovskite solar cells[J].Science,2018,361(6408):8235-1-7.
[3] Sha W E I,Ren X,Chen L,et al.The efficiency limit of CH3NH3PbI3 perovskite solar cells[J].Applied Physics Letters,2015,106(22):221104-1-5.
[4] Im J H,Kim H S,Park N G.Morphology-photovoltaic property correlation in perovskite solar cells:one-step versus two-step deposition of CH3NH3PbI3[J].APL Materials,2014,2(8):081510-1-8.
[5] Jeng J Y,Chiang Y F,Lee M H,et al.CH3NH3PbI3 perovskite/fullerene planar-heterojunction hybrid solar cells[J].Advanced Materials,2013,25(27):3727-3732.
[6] Kojima A,Teshima K,Shirai Y,et al.Organometal halide perovskites as visible-light sensitizers for photovoltaic cells[J].Journal of the American Chemical Society,2009,131(17):6050-6051.
[7] Kim G H,Kim D S.Development of perovskite solar cells with >25% conversion efficiency[J].Joule,2021,5(5):1033-1035.
[8] Chen Z,Wang J J,Ren Y,et al.Schottky solar cells based on CsSnI3 thin-films[J].Applied Physics Letters,2012,101(9):093901-1-4.
[9] Hu Y,Bai F,Liu X,et al.Bismuth incorporation stabilized α-CsPbI3 for fully inorganic perovskite solar cells[J].ACS Energy Letters,2017,2(10):2219-2227.
[10] Wang Y,Dar M I,Ono L K,et al.Thermodynamically stabilized β-CsPbI3-based perovskite solar cells with efficiencies >18%[J].Science,2019,365(6453):591-595.
[11] Tong G,Chen T,Li H,et al.Phase transition induced recrystallization and low surface potential barrier leading to 10.91%-efficient CsPbBr3 perovskite solar cells[J].Nano Energy,2019,65:104015-1-10.
[12] Ghaithan H M,Alahmed Z A,Qaid S M H,et al.First principle-based calculations of the optoelectronic features of 2×2×2 CsPb(I1-xBrx)3 perovskite[J].Superlattices and Microstructures,2020,140:106474-1-18.
[13] Yang P,Liu P,Ullah S,et al.The investigation of CsPb(I1-xBrx)3 crystalline silicon two-and four-terminal tandem solar cells[J].Solar Energy,2021,216:145-150.
[14] Ghaithan H M,Alahmed Z A,Lyras A,et al.Computational investigation of the folded and unfolded band structure and structural and optical properties of CsPb(I1-xBrx)3 perovskites[J].Crystals,2020,10(5):342-1-14.
[15] Kulbak M,Cahen D,Hodes G.How important is the organic part of lead halide perovskite photovoltaic cells? efficient CsPbBr3 cells[J].The Journal of Physical Chemistry Letters,2015,6(13):2452-2456.
[16] Wang P,Zhang X,Zhou Y,et al.Solvent-controlled growth of inorganic perovskite films in dry environment for efficient and stable solar cells[J].Nature Communications,2018,9(1):1-7.
[17] Zhao Y,Duan J,Yuan H,et al.Using SnO2 QDs and CsMBr3 (M=Sn,Bi,Cu) QDs as charge-transporting materials for 10.6%-efficiency all-inorganic CsPbBr3 perovskite solar cells with an ultrahigh open-circuit voltage of 1.610V[J].Solar Rrl,2019,3(3):1800284-1-7.
[18] Liu Y,Xiang T,Zhang B,et al.Defect passivation and fermi level modification for >10% evaporated all-inorganic CsPbBr3 perovskite solar cells[J].ACS Applied Energy Materials,2022,5(7):8049-8056.
[19] Mehrabian M,Afshar E N,Yousefzadeh S A.Simulating the thickness effect of the graphene oxide layer in CsPbBr3-based solar cells[J].Materials Research Express,2021,8(3):035509-1-7.
[20] Zhou Z J,Deng Y Q,Zhang P P,et al.Cu2ZnSnS4 quantum dots as hole transport material for enhanced charge extraction and stability in all-inorganic CsPbBr3 perovskite solar cells[J].Solar Rrl,2019,3(4):1800354-1-6.
[21] Rahman M A.Design and simulation of a high-performance Cd-free Cu2SnSe3 solar cells with SnS electron-blocking hole transport layer and TiO2 electron transport layer by SCAPS-1D[J].SN Applied Sciences,2021,3(2):1-15.
[22] Slami A,Bouchaour M,Merad L.Numerical study of based perovskite solar cells by SCAPS-1D[J].International Journal of Energy and Environment (IJEE),2019,13:17-21.
[23] Ullah S,Liu P,Wang J,et al.Optimizing the working mechanism of the CsPbBr3-based inorganic perovskite solar cells for enhanced efficiency[J].Solar Energy,2020,209:79-84.
[24] Djinkwi Wanda M,Ouédraogo S,Tchoffo F,et al.Numerical investigations and analysis of Cu2ZnSnS4 based solar cells by SCAPS-1D[J].International Journal of Photoenergy,2016,2016:1-10.
[25] Lin P,Lin L,Yu J,et al.Numerical simulation of Cu2ZnSnS4 based solar cells with In2S3 buffer layers by SCAPS-1D[J].Journal of Applied Science and Engineering,2014,17(4):383-390.
[26] Xosrovashvili G,Gorji N E.Numerical analysis of TiO2/Cu2ZnSnS4 nanostructured PV using SCAPS-1D[J].Journal of Modern Optics,2013,60(11):936-940.
[27] Lin P,Lin L,Yu J,et al.Numerical simulation of Cu2ZnSnS4 based solar cells with In2S3 buffer layers by SCAPS-1D[J].Journal of Applied Science and Engineering,2014,17(4):383-390.

基金资助

兴义民族师范学院重大项目(21XYZD09);兴义民族师范学院博士基金(23XYBS17);黔西南州科技局科技计划(2021-2-37);兴义民族师范学院教授科研基金(19XYJS05);贵州省教育厅拔尖人才项目(黔科教[2022]094)

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