固体氧化物电解池电解CO2阴极材料进展

杨浦1,2, 刘菲1,2, 邵天琦1,2, 董润泽1,2, 李萍1,2*, 付东1,2

化工新型材料 ›› 2023, Vol. 51 ›› Issue (2) : 249 -253.

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化工新型材料 ›› 2023, Vol. 51 ›› Issue (2) : 249-253. DOI: 10.19817/j.cnki.issn1006-3536.2023.02.050
开发与应用

固体氧化物电解池电解CO2阴极材料进展

    杨浦1,2, 刘菲1,2, 邵天琦1,2, 董润泽1,2, 李萍1,2*, 付东1,2
作者信息 +

Development of cathode materials for CO2 electrolysis in solid oxide electrolysis cell

  • Yang Pu1,2, Liu Fei1,2, Shao Tianqi1,2, Dong Runze1,2, Li Ping1,2, Fu Dong1,2
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摘要

为了实现可持续发展的未来,固体氧化物电解电池(SOECs)作为一种结合二氧化碳还原和可再生能源利用的高效技术越来越具吸引力。综述了目前常用的SOEC电解CO2的阴极材料,包括金属氧化物、钙钛矿、双钙钛矿型以及原位析出金属/合金型阴极材料的相关研究工作,并探究了CO2电解的阴极反应机理,以期为后续阴极材料的研究提供思路。

Abstract

In order to achieve sustainable development,solid oxide electrolysis cells (SOECs) are becoming more and more attractive as a high-efficiency technology that combines carbon dioxide reduction and renewable energy utilization.This article reviewed commonly used cathode materials for SOEC electrolysis of CO2,including metal oxides,perovskite oxides,double perovskite oxides,and phase-transformation in-situ precipitation metal/alloy cathode materials.The cathode reaction mechanism of CO2 electrolysis was explored in order to provide ideas for subsequent cathode materials research.

关键词

二氧化碳 / 固体氧化物电解池 / 阴极 / 钙钛矿

Key words

carbon dioxide / solid oxide electrolysis cell / cathode / perovskite

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固体氧化物电解池电解CO2阴极材料进展[J]. 化工新型材料, 2023, 51(2): 249-253 DOI:10.19817/j.cnki.issn1006-3536.2023.02.050

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基金资助

国家自然科学基金(52102246);中央高校基本科研业务费专项资金(2020MS124和2020MS126);河北省自然科学基金项目(B2020502002和B2020502003)

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