综述与专论

我国PPCPs污染与治理技术研究进展

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  • 1.吉林师范大学吉林省高校环境材料与污染控制重点实验室,四平136000;
    2.吉林师范大学环境科学与工程学院,四平136000
吕文静(1996-),女,硕士研究生,主要研究方向为污废水高级氧化处理。

收稿日期: 2019-04-19

  修回日期: 2019-11-12

  网络出版日期: 2020-10-23

基金资助

国家自然科学基金(5170081750);吉林省靶向识别与光催化降解材料科技创新中心(20180623042TC);吉林省教育厅项目(JJKH20180790KJ)

Research progress of PPCPs pollution and treatment technology in China

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  • 1. Key Laboratory of Environmental Materials and Pollution Control,the Education Department of Jilin Province,Jilin Normal University,Siping 136000;
    2. College of Environmental Science and Engineering,Jilin Normal University,Siping 136000

Received date: 2019-04-19

  Revised date: 2019-11-12

  Online published: 2020-10-23

摘要

药品和个人护理品(PPCPs)是一类对人类健康和生态安全构成潜在危害的新型微量有机污染物,尽管在水体中的浓度很低,但由于其结构复杂、难生物降解、在环境中呈伪持续存在状态等特点而对水环境产生深远影响。简要说明了PPCPs对生物和环境的危害、我国PPCPs污染现状,以及处理PPCPs的各种方法,重点介绍了生物处理法、物理化学方法和高级氧化技术等的研究进展,分析了各种方法在废水处理中的优势和缺点,并展望了未来降解处理PPCPs的研究方向。

本文引用格式

吕文静, 朱琳, 孔祥权, 杨春维 . 我国PPCPs污染与治理技术研究进展[J]. 化工新型材料, 2020 , 48(8) : 42 -45 . DOI: 10.19817/j.cnki.issn 1006-3536.2020.08.009

Abstract

Pharmaceutical and personal care products (PPCPs) are a new class of trace organic contaminants that pose a potential hazard to human health and ecological safety.Although their concentration in water is low,they are complex,difficult to biodegrade,and with pseudo-persistent state in the environment.The characteristics of pseudo-persistent state is under a profound impact on the water environment.The biological and environmental hazards of PPCPs,the current status of PPCPs pollution in China,and various methods for treating PPCPs were briefly described.The research progress in the removal of PPCPs from water,such as biological treatment,physical and chemical methods and advanced oxidation technology were introduced.The advantages and disadvantages of the methods in wastewater treatment were studied,and predicated the future research directions of degradation treatment of PPCPs.

参考文献

[1] Soohyung P,Wontae L.Removal of selected pharmaceuticals and personal care products in reclaimed water during simulated managed aquifer recharge[J].Science of The Total Environment,2018,640-641:671-677.
[2] Papa E,Sangion A,Arnot J A,et al.Development of human biotransformation QSARs and application for PBT assessment refinement[J].Food and Chemical Toxicology,2017,112.
[3] Rubasinghege G,Gurung R,Rijal H,et al.Abiotic degradation and environmental toxicity of ibuprofen:roles of mineral particles and solar radiation[J].Water Research,2018,131:22-32.
[4] Chen Y,Xu W,Zhu H,et al.Comparison of organic matter removals in single-component and bi-component systems using enhanced coagulation and magnetic ion exchange (MIEX) adsorption[J].Chemosphere.2018,210:672-682.
[5] Ali A M,Rønning H T,Sydnes L K,et al.Detection of PPCPs in marine organisms from contaminated coastal waters of the Saudi Red Sea[J].The Science of The Total Environment,2018,621:654-662.
[6] Li Q,Zhang Y,Lu Y,et al.Risk ranking of environmental contaminants in Xiaoqing River,a heavily polluted river along urbanizing Bohai Rim[J].Chemosphere,2018,204:28-35.
[7] Sakalli S,Giang P T,Burkina V,et al.The effects of sewage treatment plant effluents on hepatic and intestinal biomarkers in common carp (Cyprinus carpio)[J].Science of the Total Environment,2018,635:1160-1169.
[8] Pusceddu F H,Choueri R B,Pereira C D S,et al.Environmental risk assessment of triclosan and ibuprofen in marine sediments using individual and sub-individual endpoints[J].Environmental Pollution,2018,232:274-283.
[9] Baron P A,Love D C,Nachman K E.Pharmaceuticals and personal care products in chicken meat and other food animal products:a market-basket pilot study[J].Science of The Total Environment,2014,490:296-300.
[10] Done H Y,Halden R U.Reconnaissance of 47 antibiotics and associated microbial risks in seafood sold in the United States[J].Journal of Hazardous Materials,2015,282:10-17.
[11] Pan M,Wong C K C,Chu L M.Distribution of antibiotics in wastewater-irrigated soils and their accumulation in vegetable crops in the Pearl River Delta,southern China[J].Journal of Agricultural and Food Chemistry,2014,62(46):11062-11069.
[12] Wilkinson J L,Hooda P S,Swinden J,et al.Spatial (bio)accumulation of pharmaceuticals,illicit drugs,plasticisers,perfluorinated compounds and metabolites in river sediment,aquatic plants and benthic organisms[J].Environmental Pollution,2018,234:864-875.
[13] 孟霞.水环境中PPCPs的处理方法及研究进展[J].城市建设理论研究(电子版),2017(20):220.
[14] Zepon Tarpani R R,Azapagic A.Life cycle environmental impacts of advanced wastewater treatment techniques for removal of pharmaceuticals and personal care products (PPCPs)[J].Journal of Environmental Management,2018,215:258-272.
[15] 高月,李杰,许楠,等.汉江水相和沉积物中药品和个人护理品(PPCPs)的污染水平与生态风险[J].环境化学,2018,37(08):1706-1719.
[16] 张盼伟,周怀东,赵高峰,等.太湖表层沉积物中PPCPs的时空分布特征及潜在风险[J].环境科学,2016,37(09):3348-3355.
[17] Li W L,Zhang Z,Ma W L,et al.An evaluation on the intra-day dynamics,seasonal variations and removal of selected pharmaceuticals and personal care products from urban wastewater treatment plants[J].Science of the Total Environment,2018,640-641:1139.
[18] Mei X,Sui Q,Lyu S,et al.Pharmaceuticals and personal care products in the urban river across the megacity Shanghai:occurrence,source apportionment and a snapshot of influence of rainfall[J].Journal of Hazardous Materials.2018,359:429-436.
[19] Ma X Y,Li Q,Wang X C,et al.Micropollutants removal and health risk reduction in a water reclamation and ecological reuse system[J].Water Research,2018,138:272-281.
[20] 康杜.生物膜光反应器去除污水中营养盐和药品及个人护理品的研究[D].北京:中国地质大学,2018.
[21] Li A,Wu Z,Wang T,et al.Kinetics and mechanisms of the degradation of PPCPs by zero-valent iron (Fe°) activated peroxydisulfate (PDS) system in groundwater[J].Journal of Hazardous Materials.2018,357:207-216.
[22] Guo X,Yin Y,Yang C,et al.Maize straw decorated with sulfide for tylosin removal from the water[J].Ecotoxicology and Environmental Safety,2018,152:16-23.
[23] Lin Y Y,Kurniawan T A,Albadarin A B,et al.Enhanced removal of acetaminophen from synthetic wastewater using multi-walled carbon nanotubes (MWCNTs) chemically modified with NaOH,HNO3/H2SO4,ozone,and/or chitosan[J].Journal of Molecular Liquids.2018,251:369-377.
[24] Li Z,Liu G,Su Q,et al.Kinetics and thermodynamics of NPX adsorption by γ-FeOOH in aqueous media[J].Arabian Journal of Chemistry.2018,11(6):910-917.
[25] Wang Y,Liu Y,Yu Y,et al.Influence of CNT-rGO composite structures on theirpermeability and selectivity for membrane water treatment[J].Journal of Membrane Science,2018,551:326-332.
[26] Li J,Zhou Q,Campos LC.The application of GAC sandwich slow sand filtration to remove pharmaceutical and personal care products[J].Science of the Total Environment.2018,635:1182-1190.
[27] Awfa D,Ateia M,Fujii M,et al.Photodegradation of pharmaceuticals and personal care products in water treatment using carbonaceous-TiO2,composites:a critical review of recent literature[J].Water Research,2018,142:26-45.
[28] Boena Czech,Tyszczuk-Rotko K.Visible-light-driven photocatalytic removal of acetaminophen from water using a novel MWCNT-TiO2-SiO2 photocatalysts[J].Separation & Purification Technology,2018,206:343-355.
[29] Kurniawan T A,Yanyan L,Ouyang T,et al.BaTiO3/TiO2 composite-assisted photocatalytic degradation for removal of acetaminophen from synthetic wastewater under UV-Vis irradiation[J].Materials Science in Semiconductor Processing.2018,73:42-50.
[30] Fan G D,Zheng X M,Luo J,et al.Rapid synthesis of Ag/AgCl@ZIF-8 as a highly efficient photocatalyst for degradation of acetaminophen under visible light[J].Chemical Engineering Journal,2018,351:782-790.
[31] Wang W,Lu Y,Luo H,et al.A microbial electro-Fenton cell for removing carbamazepine in wastewater with electricity output[J].Water Research,2018,139:58-65.
[32] Yang H,Zhou M,Yang W,et al.Rolling-made gas diffusion electrode with carbon nanotube for electro-Fenton degradation of acetylsalicylic acid[J].Chemosphere,2018,439-446
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