Preparation of Zn-P/GO composite and its photodegradation of methylene blue

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  • College of Chemistry,Changchun Normal University,Changchun 130032

Received date: 2020-08-12

  Revised date: 2021-06-21

  Online published: 2021-09-30

Abstract

A novel zinc porphyrin and graphene oxide (Zn-P/GO) composite was prepared by combining long chain tetra (3,5-dimethoxyl-4-myristoyloxy)phenyl porphyrin zinc (Zn-P) with graphene oxide (GO).The results of SEM,UV-Vis and IR shown that the binding mode of Zn-P and GO was non covalent bond-stacking.In order to study the photodegradation performance of Zn-P/GO,methylene blue (MB) was selected as the model organic pollutant to study the catalytic degradation efficiency of the composite under different light sources,and the photodegradation efficiency of Zn-P/Go and Zn-P was compared.

Cite this article

Sun Erjun, Chang Yu, Jiang Luyu, Li Siqi, Li Yansong, Wang YueSun, Guojian, Wang Shanshan . Preparation of Zn-P/GO composite and its photodegradation of methylene blue[J]. New Chemical Materials, 2021 , 49(9) : 276 -279 . DOI: 10.19817/j.cnki.issn 1006-3536.2021.09.060

References

[1] 丁绍兰,李郑坤,王睿.染料废水处理技术综述[J].水资源保护,2010,26(3):73-78.
[2] Xian M,Liu Z,Cheng D,et al.Microporous nano-MgO/diatomite ceramic membrane with high positive surface charge for tetracycline removal[J].Journal of Hazardous Materials,2016,320(15):495-503.
[3] Mu B,Wang A.Adsorption of dyes onto palygorskite and its composites:a review[J].Journal of Environmental Chemical Engineering,2016,4(1):1274-1294.
[4] 曹婷婷,邹彩琼,罗光富,等.非水溶性席夫碱铁疏水异相光催化降解有毒有机污染物[J].高等学校化学学报,2011,32(1):105-112.
[5] 杨卫军,张静余,严敏鸣.亚甲基蓝检测方法及代谢动力学研究进展[J].食品安全质量检测学报,2018,9(10):2419-2425.
[6] 单斌,王安琪,魏霄飞,等.TiO2型光催化剂在染料废水处理中的应用进展[J].染料与染色,2018,55(6):55-60.
[7] 李福颖,郑俊垲,牛玉,等.TiO2/氧化石墨烯光催化降解亚甲基蓝性能研究[J].化学研究与应用,2019,31(6):1167-1172.
[8] 孟祖超,刘斌,李成希,等.金属-有机骨架复合材料Cu-1,3,5-苯三甲酸/氧化石墨烯对亚甲基蓝的吸附性能研究[J].化工新型材料,2018,46(11):225-229.
[9] 袁秋兰,项小燕,吴亮亮,等.四(对-磺酸基苯基)卟啉催化降解亚甲基蓝染料废水[J].化学工程与装备,2011(3):174-177.
[10] 赵晓娜,张鹏,赵义斐,等.金属卟啉衍生物催化降解污染物研究进展[J].环境化学,2019,38(9):2067-2080.
[11] 刘洋洋,顾宝珊,郑艳银,等.氧化石墨烯对亚甲基蓝的可见光催化降解[J].化工新型材料,2019,47(3):211-215.
[12] 郑艳银,顾宝珊,孙世清,等.改性石墨烯光催化薄膜的制备及可见光光催化性能[J].材料科学与工程学报,2019,37(2):250-256,285.
[13] 韩雅楠,张宝,冯亚青.铁-锌卟啉框架材料及其可见光催化降解罗丹明[J].精细化工,2019,36(7):1428-1433,1482.
[14] 李营营.氧化石墨烯与锰卟啉复合物的制备及其催化性能研究[D].长沙:湖南大学,2018.
[15] Huang D K,Lu J F,Li S H,et al.Fabrication of cobalt porphyrin,electrochemically resuced gtaphene oxide hybrid films foe electrocatalytic hydrogen evolution in aqueous solution[J].Langmuir,2014,30(23):6990-6998.
[16] 孙二军,王珊珊,白晓燕,等.长链卟啉金属配合物的合成与性质研究[J].合成化学,2020,28(7):620-625.
[17] 陈国良.类石墨烯-卟啉二维纳米复合材料的制备及其光电催化性能研究[D].长沙:湖南科技大学,2017.
[18] 孙国建.长链卟啉—石墨烯复合材料的合成、光电性质及应用研究[D].长春:长春师范大学,2020.
[19] 杜慧琳.石墨烯/卟啉复合物的电化学及光电性能[D].太原:山西大学,2015.
[20] 万军民.四苯基卟啉衍生物光诱导电子转移动力学及其敏化TiO2可见光催化染料的研究[D].杭州:浙江理工大学,2011.
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