Please wait a minute...
 首页  期刊简介 期刊订阅 广告合作 联系我们
 
最新录用  |  当期目录  |  过刊浏览  |  热点文章  |  阅读排行
化工新型材料  2019, Vol. 47 Issue (11): 222-226    
  开发与应用 本期目录 | 过刊浏览 | 高级检索 |
氧化石墨烯薄膜的制备及其吸附PM2.5性能研究
邹卫武1,2, 顾宝珊2*, 孙世清1, 王仕东1,2, 李鑫2, 赵皓琦2
1.河北科技大学材料科学与工程学院,石家庄050000;
2.中国钢研科技集团有限公司先进金属材料涂镀国家工程实验室,北京100081
Preparation of GO film and their adsorption property for PM2.5
Zou Weiwu1,2, Gu Baoshan2, Sun Shiqing1, Wang Shidong1,2, Li Xin2, Zhao Haoqi2
1.School of Materials Science and Engineering,Hebei University of Science and Technology,Shijiazhuang 050000;
2.National Engineering Laboratory for Advanced Coatings Technology of Metal Materials,China Iron and Steel Research Institute Group,Beijing 100081
下载:  PDF (5283KB) 
输出:  BibTeX | EndNote (RIS)      
摘要 为探究氧化石墨烯(GO)对PM2.5的吸附性能,采用喷涂方式,制备了以4种不同无纺布为基底的GO薄膜,测试了其吸附性能及薄膜长效性。采用扫描电镜、拉曼光谱、X射线衍射及红外光谱进行表征。结果表明:GO成功附着在无纺布纤维表面及纤维间形成薄膜,并且GO材料存在对PM2.5的吸附性且效果明显。不同基底上GO薄膜去除率分别约为34%、95%、45%及82%,提高了27%、5%、30%及28%。经过15d的连续测量,GO薄膜对PM2.5的去除保持了良好的稳定性及长效性。
服务
把本文推荐给朋友
加入引用管理器
E-mail Alert
RSS
作者相关文章
邹卫武
顾宝珊
孙世清
王仕东
李鑫
赵皓琦
关键词:  氧化石墨烯  薄膜  PM2.5  吸附    
Abstract: In order to investigate the adsorption properties of graphene oxide (GO) on PM2.5,GO films based on four different non-woven fabrics were prepared by spraying method,and their adsorption properties and long-term effectiveness were tested.The samples were characterized by scanning electron microscopy,raman spectroscopy,X-ray diffraction and Infrared spectroscopy.The results shown that GO was adhered to the surface of the non-woven fabric and formed a film between the fibers.The GO material had the adsorption property to PM2.5 and the effect was obvious.The GO film removal efficiency on different substrates were 34%,95%,45%,and 82%,respectively,which increased by 27%,5%,30%,and 28%.After 15 days of continuous measurement,the removal of PM2.5 by GO film maintained good stability and long-term effectiveness.
Key words:  graphene oxide    film    PM2.5    adsorption
收稿日期:  2019-05-22                出版日期:  2019-11-20      发布日期:  2019-12-04      期的出版日期:  2019-11-20
基金资助: 河北科技大学科学治霾及大气污染防治重点攻关预研专项课题(10)
通讯作者:  顾宝珊,教授。   
作者简介:  邹卫武(1993-),男,硕士研究生,主要从事石墨烯净化空气的研究。
引用本文:    
邹卫武, 顾宝珊, 孙世清, 王仕东, 李鑫, 赵皓琦. 氧化石墨烯薄膜的制备及其吸附PM2.5性能研究[J]. 化工新型材料, 2019, 47(11): 222-226.
Zou Weiwu, Gu Baoshan, Sun Shiqing, Wang Shidong, Li Xin, Zhao Haoqi. Preparation of GO film and their adsorption property for PM2.5. New Chemical Materials, 2019, 47(11): 222-226.
链接本文:  
https://www.hgxx.org/CN/  或          https://www.hgxx.org/CN/Y2019/V47/I11/222
[1] Zhang R,Liu C,Hsu P C,et al.Nanofiber air filters with high-temperature stability for efficient PM2.5 removal from the pollution sources[J].Nano Letters,2016,16(6):3642.
[2] Wang Q,Bai Y,Xie J,et al.Synthesis and filtration properties of polyimide nanofiber membrane/carbon woven fabric sandwiched hot gas filters for removal of PM2.5 particles[J].Powder Technology,2016,292:54-63.
[3] Xu J,Liu C,Hsu P C,et al.Roll-to-roll transfer of electrospun nanofiber film for high-efficiency transparent air filter[J].Nano Letters,2016,16(2):1270.
[4] Kchristian K,Humaira S,Muhammad S,et al.Environmental applications using graphene composites:water remediation and gas adsorption[J].Nanoscale,2013,5(8):3149-3171.
[5] Liu B,Zhang S,Wang X,et al.Efficient and reusable polyamide-56 nanofiber/nets membrane with bimodal structures for air filtration[J].Journal of Colloid & Interface Science,2015,457:203-211.
[6] Chen R,Zhang X,Wang P,et al.Transparent thermoplastic polyurethane air filters for efficient electrostatic capture of particulate matter pollutants[J].Nanotechnology,2018,30(1):15703.
[7] Liu C,Hsu P C,Lee H W,et al.Transparent air filter for high-efficiency PM2.5 capture[J].Nature Communications,2015,6:6205.
[8] Lian T,Li Y,Ye C,et al.Preparation and characterization of graphene reinforced PA6 fiber[J].Journal of Applied Polymer Science,2017,135(10):45834.
[9] Balandin A A,Ghosh S,Bao W,et al.Superior thermal conductivity of single-layer graphene[J].Nano Letters,2008,8(3):902.
[10] Yanwu Z,Shanthi M,Weiwei C,et al.Graphene and graphene oxide:synthesis,properties,and applications[J].Cheminform,2010,22(35):3906-3924.
[11] Jing B,Nan H,Han Q,et al.The Effect of Au nanoparticles on the strain-dependent electrical properties of cvd graphene[J].Journal of Nanoparticle Research,2018,20(3):69.
[12] Yoo B M,Shin J E,Lee H D,et al.Graphene and graphene oxide membranes for gas separation applications[J].Current Opinion in Chemical Engineering,2017,16:39-47.
[13] Jr W S H,Offeman R E.Preparation of graphitic oxide[J].J Am Chem Soc,1958,80(6):1339.
[14] 刘洋洋,顾宝珊,郑艳银,等.氧化石墨烯对亚甲基蓝的可见光催化降解[J].化工新型材料,2019,47(3):211-215.
[15] 刘洋洋,顾宝珊,郑艳银,等.氧化石墨烯可见光催化能力的影响因素[J].材料科学与工艺,2018,26(4):80-87.
[16] 刘洋洋.氧化石墨烯光催化机理及在污水处理领域应用[D].北京:钢铁研究总院,2017.
[17] 郑艳银.石墨烯净化城市污水技术与机理研究[D].石家庄:河北科技大学,2018.
[18] Zhang X,Zhang W,Yi M,et al.High-performance inertial impaction filters for particulate matter removal[J].Sci Rep,2018,8(1):4757.
[19] 邹卫武.一种测量石墨烯薄膜空气净化性能的装置:中国201821650411.5[P].2019-06-28.
[20] Jing L,Zhang D,Yang T,et al.Nanofibrous membrane of graphene oxide-in-polyacrylonitrile composite with low filtration resistance for the effective capture of PM2.5[J].Journal of Membrane Science,2018,551:85-92.
[21] Liang J,Cai Z,Li L,et al.Scalable and facile preparation of graphene aerogel for air purification[J].Rsc Advances,2014,4(10):4843-4847.
[1] 时雅滨, 许晓娟, 贾启华, 高丹, 田明, 孙丽, 宋广凤, 张学彬. 层层自组装技术制备新型功能高分子材料研究进展[J]. 化工新型材料, 2019, 47(9): 11-13.
[2] 董玲玉, 张婷, 钱春园. 凹凸棒石基复合材料制备研究进展[J]. 化工新型材料, 2019, 47(9): 14-18.
[3] 王爽, 许国根, 贾瑛, 王坤. 改性海藻酸钠凝胶球的制备及去除偏二甲肼研究[J]. 化工新型材料, 2019, 47(9): 178-181.
[4] 张彦平, 程恒卫, 路广平, 张越. 钡改性污泥陶粒对废水中Cr(Ⅵ)的吸附性能研究[J]. 化工新型材料, 2019, 47(9): 195-198.
[5] 吴鸣, 高跃, 王旺成, 孙红梅, 彭啸, 吴燕. 石墨烯/SiO2复合气凝胶微球的制备及其吸附性能研究[J]. 化工新型材料, 2019, 47(9): 155-160.
[6] 李胜英, 郭呈若, 李春娴, 陈慧文, 符永婷, 冯建海. Zn-MOF前驱法制备ZnO/TiO2及其吸附降解性能[J]. 化工新型材料, 2019, 47(9): 166-169.
[7] 刘雪梅, 马闯, 吴凡, 赵蓓. 异介质甘蔗渣基水热炭对Cr(Ⅵ)的吸附特性[J]. 化工新型材料, 2019, 47(9): 215-219.
[8] 王攀峰, 邰文亮, 杨贤, 王强, 花榕, 刘云海. 改性甘蔗渣吸附水中Th(Ⅳ)的研究[J]. 化工新型材料, 2019, 47(9): 174-177.
[9] 王娇娜, 潘思博, 王其智, 漆麟, 李凤飞, 方亦男, 李秀艳. 静电纺-LbL技术制备[CTS/SA]c/lPVA纳米复合膜及其性能研究[J]. 化工新型材料, 2019, 47(8): 94-98.
[10] 袁艺, 李泽晖, 王亚玲, 刘星辰, 吴晓雪, 蒋靖坤. 金属-有机骨架材料对环境中典型苯系物的吸附研究进展[J]. 化工新型材料, 2019, 47(8): 18-22.
[11] 吴炎森, 许佳佳, 李旭娇, 唐丽永. 层层浸渍法制备Eu3+∶KY(WO4)2薄膜及其发光性能研究[J]. 化工新型材料, 2019, 47(8): 49-52.
[12] 鲍田, 王东. 溶胶-凝胶法AZO/rGO薄膜的制备研究[J]. 化工新型材料, 2019, 47(8): 102-105.
[13] 张毅, 高园园, 张昊, 周省, 刘叶. 改性淀粉微球对废水中Cu2+、Ni2+吸附性能的研究[J]. 化工新型材料, 2019, 47(8): 190-192.
[14] 盛盼盼, 孙富安, 陈乐, 张致慧, 何明阳. ZIF-8负载离子交换树脂复合材料对铀酰的吸附行为研究[J]. 化工新型材料, 2019, 47(8): 256-260.
[15] 谢新玲, 黄婕, 张友全, 秦祖赠, 廖安平. 改性磁性木薯渣微球的制备及对Pb(Ⅱ)的吸附[J]. 化工新型材料, 2019, 47(8): 158-162.
[1] Li Chunjing, Yang Ruixia, Ma Hao, Jin Huijiao, Shi Xiaodong, Ma Wenjing. Preparation of CH3NH3PbI2Br light absorber-layer thin film[J]. New Chemical Materials, 2018, 46(2): 155 -159 .
[2] Qiu Zhiwen, Sun Xiaogang, Pang Zhipeng, Liu Zhenhong, Chen Long, Cai Manyuan. Study on EMI shielding performance of conductive paper doped with carbon nanotube and rare earth oxide[J]. New Chemical Materials, 2018, 46(3): 75 -79 .
[3] Su Wei, Ran Meng, Zhang Ai, Sun Yan. Preparation of sulfur-doped microporous carbon and its adsorption property[J]. New Chemical Materials, 2018, 46(4): 161 -164 .
[4] Bao Huashan, Wang Erjing, Song Chengjie, Wang Shimin. Research progress of thermally activated delayed fluorescence emitter and device based on small organic molecule[J]. New Chemical Materials, 2018, 46(5): 7 -10 .
[5] Wang Yufei, Zheng Liping, Yao Jianhua, Li Jingjing. Novel progress of fluorofullerene applied in electronic material and device[J]. New Chemical Materials, 2018, 46(7): 5 -8 .
[6] Su Yan, Zhang Qiang, Wang Bei, Deng Wei, Liang Yingchun, Yang Chaolong, Li Youbing. Preparation of PVA red-light film and research on its property[J]. New Chemical Materials, 2018, 46(9): 77 -79 .
[7] Geng Siyao, Wang Jie, Yao Bolong, Wang Likui. Synthesis and property of UV-curable fluorine-containing hyperbranched polyurethane[J]. New Chemical Materials, 2019, 47(1): 100 -104 .
[8] Shi Suyu, Ren Jiahua, Wang Lina, Xie Xiaokai, Xin Changzheng. Preparation and characterization of CS anion-exchange membrane modified by TPU conductive nonwoven[J]. New Chemical Materials, 2019, 47(2): 136 -139 .
[9] Wang Yuanhang, Zhang Naien, Guo Xiaorong, Yan Hong. Progress of intumescent flame retardant coating on material surface[J]. New Chemical Materials, 2019, 47(6): 39 -43 .
Viewed
Full text


Abstract

Cited

  Shared   
  Discussed   
京ICP备09035943号-38
版权所有 © 《化工新型材料》编辑部
本系统由北京玛格泰克科技发展有限公司设计开发 技术支持:support@magtech.com.cn